In an antibiotic degradation experiment using metals carbon composites to activate PMS, the results doesn't fit pseudo first or second order kinetics however the degradation efficiency is very high during the first 10 min.
Dr Manzoor Ahmed Sanjrani Muhammad Muneeb Ur Rehman Pablo K. Cornejo Dr K N Sheth
While the basic problem is vastly different, the answer is the same as the one here:
https://www.researchgate.net/post/Why_reaction_order_is_changing_with_temperature_Is_it_a_non_elementary_reaction
You are facing a complex reaction with many elemental steps, each of which has its own rate coefficient. Depending on the current concentration, different components may e.g. be assumed quasi-stationary or quasi-equilibrated, so the changes in behaviour may change severely.
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