Determining the binary layer structure of Urea derived Carbon Nitride (UCN) involves a few steps:

1. **Synthesis**: UCN can be synthesized through the pyrolysis of urea under ambient pressure without additive assistance¹.

2. **Characterization**: After synthesis, the structure of UCN can be characterized using various techniques. These may include X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FTIR), and X-ray photoelectron spectroscopy (XPS)².

3. **Microscopy**: Techniques such as transmission electron microscopy (TEM) and scanning electron microscopy (SEM) can be used to visualize the binary layer structure³.

4. **Analysis**: The data obtained from these techniques can be analyzed to determine the binary layer structure of UCN³.

Remember, the specifics of your experimental design might need to be adjusted based on the characteristics of the UCN and the specific objectives of your research. It's always a good idea to consult with a materials scientist or chemist to ensure your experimental design is robust and appropriate for your study.

(1) Simple pyrolysis of urea into graphitic carbon nitride with recyclable .... https://pubs.rsc.org/en/content/articlelanding/2011/jm/c1jm12620b.

(2) Carbon nitrides: synthesis and characterization of a new class of .... https://pubs.rsc.org/en/content/articlehtml/2017/cp/c7cp02711g.

(3) Layered graphitic carbon nitride: nano-heterostructures, photo/electro .... https://link.springer.com/article/10.1007/s40097-021-00442-5.