The viscosity at infinite shear rate cannot be determined from the data shown. The viscosity curve does not show a plateau at high shear rates. Just assume its value to be zero. The viscosity at zero shear rate (etha 0) is simply the value shown in your data at zero shear.
Now make a double logarithmic plot of the viscosity versus shear rate. The slope of the curve at high shear rates now equals -m. Extrapolation of the tangent towards shear rate 0 is equal to ln(etha 0) - m ln(C).
Most of the rheology instrument softwares are powerful and can be used to fit the cross model. If you have used a ARES instrument then TRIOS software can be used for fitting the data. Just get the software and become familiar with it that's all.