I only think that fishes, being on top of the trophic chain, accumulate more heavy metals!
Thank to biomagification studies, we know that, since higher trophic levels consume more organic matter, they will accumulate more heavy metals (since they are difficult to dispose of).
I think it is depended to you that which of mollusk or fishes you want to select for your study. if you want fishes for study , benthic fishes such as halibut family very good for your survey also filter feeder mollusk has the best in between mollusk.