Can anyone direct me to papers giving the chemical reactions between hydrocarbons and water in shale gas reservoirs in the isotope reversal zone?

03 March 2016 1 2K Report

I'm looking for chemical reactions proposed for water and light hydrocarbons in the isotope and butane isomer reversal zone at high thermal maturity (> 1.5 Ro%) in shale gas reservoirs. I have papers discussing the broad concept but I'd like more details on the actual reactions proposed. Any help or further discussion would be much appreciated. Thanks, Jim

James Michael Wood

UPDATE - for those following this question, the two most relevant papers I have found so far are:

(1) Burruss, R.C. and Laughrey, C.D., 2010. Carbon and hydrogen isotopic reversals in deep basin gas: Evidence for limits to the stability of hydrocarbons. Organic Geochemistry, 41(12), pp.1285-1296.

(2) Gao, L., Schimmelmann, A., Tang, Y. and Mastalerz, M., 2014. Isotope rollover in shale gas observed in laboratory pyrolysis experiments: Insight to the role of water in thermogenesis of mature gas. Organic Geochemistry, 68, pp.95-106.

If anyone knows of other relevant papers, please let me know. Thanks, Jim

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