Internal exposures arise from the intake of terrestrial radionuclides by inhalation and ingestion. Doses by inhalation result from the presence in air of dust particles containing radionuclides of the 238Uand 232Th decay chains. The dominant component of inhalation exposure is the short-lived decay products of radon. Doses by ingestion are mainly due to 40K and to the 238U and 232Th series radionuclides present in foods and drinking water.
Yes, but as any K contains the same amount of K-40 and K is an essential element, the exposure due to internal K-40 can not be avoided by dietary measures. It will always be the same. In comparison, the uptake of U-238, Th-232 and their decay products can be influenced or avoided,
Ra is accumulated by plants in a much greater degree than U and Th because of its geochemical nature. Plants have limits on U and Th uptake, while Ra can be accumulated by plants without limits. We investigated the content of naturally occuring radionuclides (NOR) in plants near NOR-contentaining wastes and Ra concentration was linearly correlated with Ra content in soils. But the U content did not increase with U content in soils and was relatively stable.
Concerning Rn, its content varies because of changes in moisture transpiration and its measuring requires high accuracy and can be complex.
Therefore, I think Ra measuring is prefered in this case.
The total effective dose from inhalation and ingestion of terrestrial radionuclides is 310 µSv, of which 170 µSv is from 40K and 140 µSv is from the long-lived radionuclides in the uranium and thorium series.
Uranium is retained in the body primarily in the skeleton. Following intake by ingestion and inhalation, thorium is mainly deposited on bone surfaces and retained for long periods.
In my experience, the concentrations of various radionuclides (U-series) can be made using HPGe detectors with the vegetation inside a Marinelli beaker. When I worked at the BALUF in Vienna, Austria, we would clean the vegetables as if they were to be eaten; then we would puree them and pour the puree into the beaker for counting. Low background counting rooms are preferred for these types of environmental measurements. Depending on the geometry and the pureed density, one could expect efficiencies on the order of 10%.
one solution could be the Gamma spectrometry, but you need a big mass of sample and normally the MDA (Bq/kg) could be to much higher.
Other solution could be the liquid scintillation counting to measure the gross alpha and gross beta activity in sample, but i think if you want know the real concentration of Uranium, Thorium and Radium you must use a radiochemistry method; sequential separation of alla nuclide and measure by alpha spectrometry. Much expansive than Gamma and LS, but with small weight you can obtain a good results in terms of MDA and concentrations.
I don't understand why measure Radon...
Be careful with the K-40 presence if you measure the total activity.
Arguably the most sensitive method to determine U (235/8), Th (232), and Ra (226) concentration in vegetation would be by mass spectrometry. This is due to the extremely low specific activity of U and Th. And, the issues with K-40 in the sample and terrestrial / cosmic HPGe background contributions will be negated.
Whole fruit/vegetable can be muffled to ash, then the residue wet ashed in strong acid, and finally the residue brought into solution in dilute acid. This solution can be nebulized into a ICP-MS for analysis.
I think you can do this with the help of HPGe/NaI detector but you have to take care of the large mass of the samples and some calculations will do the job.
Solid state nuclear track detectors CR-39 is the preferred method to determine Radon and Uranium, also gamma ray spectroscopy to measuring Radium and Thorium.
You can measure radon and from this you can calculate the annual effective dose
by using passive technique with solid state nuclear track detectors (CR-39, LR-115,......) but if you want to determine U, Th, K you can use scintillation counter like [NaI (Tl)] and HPGe, from the results of gamma you can calculate the all kind of dose.......
*I am agreement with the answer of Dr. Olga Marinich , Dr.Ghassan Saffarini and Dr. Laith Najam and Dr. Anees A. Al-Hamzawi
Ra-226. Ra-228, K-40...u might check the Transfer Factor from the soil to plant as well together with Ingestion Dose Intake. Finally based on the UNSCEAR 2000, u might determine the Radium equivalent, annual effective dose, external hazard index.