Try the noble metals Ag/Au/Pt/ and Pd too because they have enhanced SPR (Surface Plasmon Resonance) and also have higher absorption coefficient. which are very important properties in Nano-sensors using nanoparticle.
And Pls go through literature review before deciding or finalising NP, to get a grip in the topic.....Al the best
Doped-silica nano-composite but first you should decided what is you r wavelength and what is the way of surface raman scattering is ? Fiber , prism or grating. To decided, you need to apply what you read on the tools that you have it in the lab.
Use noble metal nanoparticles for SERS, they shows surface plasmon resonance. This enhanced electric field is one important factor for increased intensity in Raman peak.